Volume 6 Issue 2
Apr.  2021
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Article Navigation >  Green Energy&Environment  > 2021  >  6(2): 212-219
Haiying Che, Xinrong Yang, Yan Yu, Chaoliang Pan, Hong Wang, Yonghong Deng, Linsen Li, Zi-Feng Ma. Engineering optimization approach of nonaqueous electrolyte for sodium ion battery with long cycle life and safety. Green Energy&Environment, 2021, 6(2): 212-219. doi: 10.1016/j.gee.2020.04.007
Citation: Haiying Che, Xinrong Yang, Yan Yu, Chaoliang Pan, Hong Wang, Yonghong Deng, Linsen Li, Zi-Feng Ma. Engineering optimization approach of nonaqueous electrolyte for sodium ion battery with long cycle life and safety. Green Energy&Environment, 2021, 6(2): 212-219. doi: 10.1016/j.gee.2020.04.007
shu

Engineering optimization approach of nonaqueous electrolyte for sodium ion battery with long cycle life and safety

doi: 10.1016/j.gee.2020.04.007
  • a.

    Shanghai Electrochemical Energy Devices Research Center, Department of Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240, China

  • b.

    Zhejiang NaTRIUM Energy Co. Ltd. Shaoxing, 312000, China

  • c.

    Shanghai Zijian Chemical Technology Co. Ltd, Shanghai, 200241, China

  • d.

    Shenzhen CAPCHEM Technology Co. Ltd, Shenzhen, 518027, China

More Information
  • Corresponding author: E-mail address: zfma@sjtu.edu.cn (Zi-Feng Ma)
  • Received date 26 February 2020, Accepted date 15 April 2020, RevRecd date 08 April 2020, Available online 25 April 2020, Publish date 30 April 2021,
    Abstract
  • Electrolyte design strategies are closely related to the capacities, cycle life and safety of sodium–ion batteries. In this study, we aimed to optimize electrolyte with the focus on engineering aspects. The basic physicochemical properties including ionic conductivity, viscosity, wettability and thermochemical stability of the electrolytes using NaPF6 as the solute and the mixed solvent with different components of EMC, DMC or DEC in PC or EC were systematically measured. Ah pouch cell with NaNi1/3Fe1/3Mn1/3O2/hard carbon electrodes was used to evaluate the performance of the prepared electrolytes. By using the Inductive Coupled Plasma Emission Spectrometer (ICP), X-ray photoelectron spectroscopy (XPS), Thermogravimetric-differential scanning calorimetry (TG-DSC) and Accelerating Rate Calorimeter (ARC), we show that an optimized electrolyte can effectively promote the formation of a protective interfacial layer on two electrodes, which not only retards parasitic reactions between the electrodes and electrolyte but also suppresses dissolution of metal ions from the cathode. With an optimized electrolyte, a NaNi1/3Fe1/3Mn1/3O2/hard carbon cell can attain 56.16% capacity retention under the low temperature of −40 °C, and can be able to retain 80% capacity retention after more than 2500 cycles while presenting excellent thermal safety.

     

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