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Yuting Zhu, Zhijing Li, Jinzhu Chen. Applications of lignin-derived catalysts for green synthesis. Green Energy&Environment, 2019, 4(3): 210-244. doi: 10.1016/j.gee.2019.01.003
Citation: Yuting Zhu, Zhijing Li, Jinzhu Chen. Applications of lignin-derived catalysts for green synthesis. Green Energy&Environment, 2019, 4(3): 210-244. doi: 10.1016/j.gee.2019.01.003
shu

Applications of lignin-derived catalysts for green synthesis

doi: 10.1016/j.gee.2019.01.003
  • a.

    Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, No. 2 Nengyuan Road, Wushan, Tianhe District, Guangzhou 510640, Guangdong, China

  • b.

    Guangdong Engineering and Technology Research Centre of Graphene-Based Materials and Products, Department of Chemistry, College of Chemistry and Materials Science, Jinan University, No. 601 Huangpu Avenue West, Tianhe District, Guangzhou 510632, Guangdong, China

  • c.

    University of Chinese Academy of Sciences, No. 19 Yuquan Road, Shijingshan District, Beijing 100049, China

  • d.

    Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Department of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, Zhejiang, China

More Information
  • Corresponding author: E-mail address: chenjz@jnu.edu.cn (Jinzhu Chen)
  • Received date 15 November 2018, Accepted date 07 January 2019, RevRecd date 07 January 2019, Available online 18 January 2019, Publish date 31 July 2019,
    Abstract
  • This review intends to introduce the application of lignin-derived catalyst for green organic synthesis over latest two decades and aims to present a renewable alternative for conventional catalyst for future industry application. The structure of lignin is initially introduced in this review. Then, various pretreatment and activation technologies of lignin are systematically presented, which includes physical activation for the formation of well-developed porosity and chemical activation to introduce catalytic active sites. Finally, the catalytic performances of various lignin-derived catalysts are rationally assessed and compared with conventional catalysts, which involves lignin-derived solid acids for hydrolysis, hydration, dehydration (trans)esterification, multi-component reaction and condensation, lignin-derived solid base for Knoevenagel reaction, lignin-derived electro-catalysts for electro-oxidation, oxygen reduction reaction, and lignin-derived supported transition metal catalysts for hydrogenation, oxidation, coupling reaction, tandem reaction, condensation reaction, ring-opening reaction, Friedel-Crafts-type reaction, Fischer–Tropsch synthesis, click reaction, Glaser reaction, cycloaddition and (trans)esterification. The above lignin-derived catalysts thus successfully promote the transformations of organic compounds, carbon dioxide, biomass-based cellulose, saccharide and vegetable oil into valuable chemicals and fuels. At the end of this review, some perspectives are given on the current issues and tendency on the lignin-derived catalysts for green chemistry.

     

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