Volume 4 Issue 4
. 
Turn off MathJax
Article Contents
Article Navigation >  Green Energy&Environment  > 2019  >  4(4): 432-438
Ling Liang, Jipeng Yan, Qian He, Tina Luong, Todd R. Pray, Blake A. Simmons, Ning Sun. Scale-up of biomass conversion using 1-ethyl-3-methylimidazolium acetate as the solvent. Green Energy&Environment, 2019, 4(4): 432-438. doi: 10.1016/j.gee.2018.07.002
Citation: Ling Liang, Jipeng Yan, Qian He, Tina Luong, Todd R. Pray, Blake A. Simmons, Ning Sun. Scale-up of biomass conversion using 1-ethyl-3-methylimidazolium acetate as the solvent. Green Energy&Environment, 2019, 4(4): 432-438. doi: 10.1016/j.gee.2018.07.002
shu

Scale-up of biomass conversion using 1-ethyl-3-methylimidazolium acetate as the solvent

doi: 10.1016/j.gee.2018.07.002
  • a.

    Advanced Biofuels and Bioproducts Process Development Unit, Lawrence Berkeley National Laboratory, Emeryville, CA, 94608, USA

  • b.

    Joint BioEnergy Institute, Lawrence Berkeley National Laboratory, Emeryville, CA, 94608, USA

More Information
  • Corresponding author: E-mail address: nsun@lbl.gov (Ning Sun)
  • Received date 26 April 2018, Accepted date 28 July 2018, RevRecd date 16 July 2018, Available online 14 August 2018, Publish date 31 October 2019,
    Abstract
  • This scale-up study demonstrated the feasibility of an ionic liquid (IL) pretreatment process at 40 kg scale, using the IL 1-ethyl-3-methylimidazolium acetate ([C2C1Im][OAc]) as the solvent. The pretreatment was followed by enzymatic hydrolysis through which the process efficiency for biomass conversion to monomeric sugars was determined. The results show that 43 wt% of switchgrass was dissolved in IL after 2 h of pretreatment at 160 °C with 15 wt% solid loading. A 120 h enzymatic hydrolysis of the pretreated switchgrass results in 96% glucan and 98% xylan conversion. [C2C1Im][OAc] pretreatment has been successfully scaled up to 40 kg with improved sugar titers and yields relative to bench scale (6 kg). The mass flow of the overall process was established and the major scale-up challenges of the process were identified.

     

    • FullText(HTML)
  • loading
    • References(44)
  • [1]
    A.Sant'Ana da Silva, S.H.Lee, T.Endo, et al. Bioresour. Technol., 102 (2011),pp. 10505-10509
    [2]
    N.Sun, M.Rahman, Y.Qin, et al. Green Chem., 11 (2009),pp. 646-655
    [3]
    V.B.Agbor, N.Cicek, R.Sparling, et al. Biotechnol. Adv., 29 (2011),pp. 675-685
    [4]
    X.Zhao, K.Cheng, D.Liu Appl. Microbiol. Biotechnol., 82 (2009),pp. 815-827
    [5]
    S.V.Farahani, Y.W.Kim, C.A.Schall Catal. Today, 269 (2016),pp. 2-8
    [6]
    A.A.Elgharbawy, M.Z.Alam, M.Moniruzzaman, et al. Biochem. Eng. J., 109 (2016),pp. 252-267
    [7]
    H.Mahmood, M.Moniruzzaman, S.Yusup, et al. J. Clean. Prod., 126 (2016),pp. 677-685
    [8]
    N.Sun, H.Liu, N.Sathitsuksanoh, et al. Biotechnol. Biofuels, 6 (2013),p. 39
    [9]
    J.A.Perez-Pimienta, M.G.Lopez-Ortega, P.Varanasi, et al. Bioresour. Technol., 127 (2013),pp. 18-24
    [10]
    G.Papa, S.Rodriguez, A.George, et al. Bioresour. Technol., 183 (2015),pp. 101-110
    [11]
    C.Li, B.Knierim, C.Manisseri, et al. Bioresour. Technol., 101 (2010),pp. 4900-4906
    [12]
    C.Li, D.Tanjore, W.He, et al. Biotechnol. Biofuels, 6 (2013),pp. 1-13
    [13]
    T. Deepti, R. Joseph, G. James, P. Paul, N. Akash, L. Chenlin, U.S. Patent No. US20160145557A1, U.S. Patent and Trademark Office, Washington, DC, 2014.
    [14]
    A.Sluiter, R.Ruiz, C.Scarlata, et al.
    [15]
    J.Yan, L.Liang, T.R.Pray, et al.
    [16]
    N.Uppugundla, L.D.C.Sousa, S.P.Chundawat, et al. Biotechnol. Biofuels, 7 (2014),p. 72
    [17]
    T.C.R.Brennan, S.Datta, H.W.Blanch, et al. Bioenergy Res., 3 (2010),pp. 123-133
    [18]
    J.Sun, J.Shi, N.V.S.N.Murthy Konda, et al. Biotechnol. Biofuels, 10 (2017),p. 154
    [19]
    M.Frederix, F.Mingardon, M.Hu, et al. Green Chem., 18 (2016),pp. 4189-4197
    [20]
    Z.Hu, R.Sykes, M.F.Davis, et al. Bioresour. Technol., 101 (2010),pp. 3253-3257
    [21]
    K.Lindsey, A.Johnson, P.Kim, et al. Biomass Bioenergy, 56 (2013),pp. 29-37
    [22]
    J.Shi, K.Balamurugan, R.Parthasarathi, et al. Green Chem., 16 (2014),pp. 3830-3840
    [23]
    J.B.Binder, R.T.Raines Proc. Natl. Acad. Sci. U. S. A., 107 (2010),pp. 4516-4521
    [24]
    X.Yuan, S.Singh, B.A.Simmons, et al. ACS Sustain. Chem. Eng., 5 (2017),pp. 4408-4413
    [25]
    D.C.Dibble, C.Li, L.Sun, et al. Green Chem., 13 (2011),pp. 3255-3264
    [26]
    M.Dimarogona, E.Topakas, L.Olsson, et al. Bioresour. Technol., 110 (2012),pp. 480-487
    [27]
    J.M.Gladden, J.I.Park, J.Bergmann, et al. Biotechnol. Biofuels, 7 (2014),pp. 15-26
    [28]
    J.I.Park, E.J.Steen, H.Burd, et al. PLoS One, 7 (2012)
    [29]
    A.G.Cruz, C.Scullin, C.Mu, et al. Biotechnol. Biofuels, 6 (2013),p. 52
    [30]
    J.Shi, V.S.Thompson, N.A.Yancey, et al. Biofuels, 4 (2013),pp. 63-72
    [31]
    F.Xu, J.Sun, N.V.S.N.M.Konda, et al. Energy Environ. Sci., 9 (2016),pp. 1042-1049
    [32]
    A.George, A.Brandt, K.Tran, et al. Green Chem., 17 (2015),pp. 1728-1734
    [33]
    C.Li, L.Liang, N.Sun, et al. Biotechnol. Biofuels, 10 (2017),p. 13
    [34]
    L.Liang, C.Li, F.Xu, et al. RSC Adv., 7 (2017),pp. 36585-36593
    [35]
    A.M.Socha, R.Parthasarathi, J.Shi, et al. Proc. Natl. Acad. Sci. U.S.A., 111 (2014),pp. E3587-E3595
    [36]
    D.Klein-Marcuschamer, P.Oleskowicz-Popiel, B.A.Simmons, et al. Biomass Bioenergy, 34 (2010),pp. 1914-1921
    [37]
    D.Klein-Marcuschamer, B.A.Simmons, H.W.Blanch Biofuels Bioprod. Biorefin., 5 (2011),pp. 562-569
    [38]
    D.Klein-Marcuschamer, C.Turner, M.Allen, et al. Biofuels Bioprod. Biorefin., 7 (2013),pp. 416-428
    [39]
    D.Klein-Marcuschamer, P.Oleskowicz-Popiel, B.A.Simmons, et al. Biotechnol. Bioeng., 109 (2012),pp. 1083-1087
    [40]
    M.Ouellet, S.Datta, D.C.Dibble, et al. Green Chem., 13 (2011),pp. 2743-2749
    [41]
    N.Nemestóthy, G.Megyeri, P.Bakonyi, et al. Bioresour. Technol., 229 (2017),pp. 190-195
    [42]
    T.L.Ruegg, E.M.Kim, B.A.Simmons, et al. Nat. Commun., 5 (2014),p. 3490
    [43]
    Q.Dickinson, S.Bottoms, L.Hinchman, et al. Microb. Cell Factories, 15 (2016),pp. 1-13
    [44]
    X.Zhong, J.Tang, L.Cao, et al. Electrochim. Acta, 244 (2017),pp. 112-118
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article views (154) PDF downloads(21) Cited by()
    Proportional views

    Publish With GEE

    Contact

    • Email：gee@ipe.ac.cn
    • Tel：010-82627075
    • Address：North 2nd street, Zhongguancun, Haidian District, Beijing, China

    Links

    京ICP备10002620号-1京公网安备 11010802039050号

    Supported by: Beijing Renhe Information Technology Co. Ltd    

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return