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Article Navigation >  Green Energy&Environment  > 2016  >  1(3): 258-265
Junfeng Wang, Camille Petit, Xiangping Zhang, Ah-Hyung Alissa Park. Simultaneous measurement of CO2 sorption and swelling of phosphate-based ionic liquid. Green Energy&Environment, 2016, 1(3): 258-265. doi: 10.1016/j.gee.2016.11.004
Citation: Junfeng Wang, Camille Petit, Xiangping Zhang, Ah-Hyung Alissa Park. Simultaneous measurement of CO2 sorption and swelling of phosphate-based ionic liquid. Green Energy&Environment, 2016, 1(3): 258-265. doi: 10.1016/j.gee.2016.11.004
shu

Simultaneous measurement of CO2 sorption and swelling of phosphate-based ionic liquid

doi: 10.1016/j.gee.2016.11.004
  • a.

    National Key Laboratory of Biochemical Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, PR China

  • b.

    Department of Earth & Environmental Engineering, Lenfest Center for Sustainable Energy, Columbia University, 500 W. 120th Street, New York, NY 10027, USA

  • c.

    Department of Chemical Engineering, Lenfest Center for Sustainable Energy, Columbia University, 500 W. 120th Street, New York, NY 10027, USA

  • d.

    Department of Chemical Engineering, Imperial College London, South Kensington Campus, London SW7 2AZ, UK

More Information
  • Corresponding author: E-mail address: junfwang@ipe.ac.cn (Junfeng Wang); E-mail address: ap2622@columbia.edu (Ah-Hyung Alissa Park)
  • Received date 29 September 2016, Accepted date 15 November 2016, RevRecd date 15 November 2016, Available online 25 November 2016, Publish date 31 October 2016,
    Abstract
  • The development of alternative CO2 capture solvents such as ionic liquids (ILs) and nanoparticle organic hybrid materials (NOHMs) have provided interesting options for CO2 capture. In this study, CO2 interactions with 1,3-dimethylimidazolium dimethylphosphate ([MMIM]DMP), 1-ethyl-3-methylimidazolium dimethylphosphate ([EMIM]DMP) and 1-ethyl-3-methylimidazolium diethylphosphate ([EMIM]DEP) that contain inorganic ester groups based on phosphate, were investigated using ATR FT-IR spectroscopy. CO2-induced swelling, CO2 diffusivity and CO2 capture capacity were simultaneously measured to identify CO2 capture mechanisms, kinetics and diffusion behaviors as a function of the alkyl chain length of the cation. Henry's law constants of CO2 were found to be in the range of 4–11 MPa, which is in agreement with those reported in other studies.

     

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