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Xueao Jiang, MingYang Xin, Long Zhao, Yang Lv, Qiyou Wang, Weijian Liu, Baoshan Xie, Yanjie Ren, Hao Li, Jian Chen. Advanced Aqueous Electrolytes toward Better Aluminum-ion Batteries: A Comprehensive Review. Green Energy&Environment. doi: 10.1016/j.gee.2026.03.013
Citation: Xueao Jiang, MingYang Xin, Long Zhao, Yang Lv, Qiyou Wang, Weijian Liu, Baoshan Xie, Yanjie Ren, Hao Li, Jian Chen. Advanced Aqueous Electrolytes toward Better Aluminum-ion Batteries: A Comprehensive Review. Green Energy&Environment. doi: 10.1016/j.gee.2026.03.013
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Advanced Aqueous Electrolytes toward Better Aluminum-ion Batteries: A Comprehensive Review

doi: 10.1016/j.gee.2026.03.013

  • 1. School of Criminal Investigation and Counter-Terrorism, Criminal Investigation Police University of China, Shenyang 110854, China;

  • 2. School of Intelligent Manufacturing and Energy Engineering, Zhejiang University of Science & Technology, Hangzhou, 310023, China;

  • 3. Key Lab for Special Functional Materials of Ministry of Education, School of Nanoscience and Materials Engineering, Henan University, Kaifeng, 475004 Henan, China;

  • 4. State Key Laboratory of Disaster Prevention & Reduction for Power Grid, Changsha University of Science & Technology, Changsha, Hunan 410014, China;

  • 5. College of Materials Science and Engineering, Hunan University, Changsha 410082, Hunan, China

Funds:

This work was financially supported by the National Natural Science Foundation of China (No. 52302242) and China Postdoctoral Science Foundation (No. 2024T170234).

  • Received date 13 November 2025, Accepted date 23 March 2026, RevRecd date 01 March 2026, Available online 01 April 2026
    Abstract
  • Rechargeable aluminium-ion batteries are emerging as promising next-generation energy storage systems, benefiting from the high mass/volumetric energy density, low cost, and intrinsic safety of Al anodes. However, their practical deployment is hindered by the limitations of conventional non-aqueous electrolytes, including moisture/oxygen sensitivity, cost, and toxicity. Aqueous aluminium-ion batteries (AAIBs) offer a compelling alternative, with advantages in cost, safety, and environmental impact. Yet, the scarcity of suitable electrolytes, particularly those capable of supporting reversible three-electron Al3+/Al redox chemistry, poses a major obstacle to commercialization. Meanwhile, developing low-cost, chemically/electrochemically stable electrolytes capable of functioning across diverse temperatures remains a critical challenge and a central research direction for advancing AAIB technology. This review comprehensively surveys advances in AAIB electrolytes, focusing on high-concentration electrolytes systems for electrochemical stability, hydrogel electrolytes that mitigate degradation through solid-phase confinement, and hydrated eutectic electrolytes for wide-temperature operation. In particular, we delve into the latest innovations in AAIB electrolyte design, provide a comprehensive perspective on current opportunities and unresolved hurdles, discuss the strengths, limitations, and potential solutions for each electrolyte type, while outline future pathways for the development of AAIB electrolytes.

     

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